Automated Author ProfileGaillardet, Jerome
Institut de physique du globe de Paris (IPGP), Paris, France0000-0001-7982-1159
Gaillardet, Jerome
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Current S-Index: 13.1 (sum of 6 datasets Dataset Index scores)
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Datasets
We provide sample information and geochemical data for obtaining erosion, weathering, and denudation rates from a framework based cosmogenic meteoric 10Be versus stable 9Be (10Be/9Be) ratios. We modified this published silicate framework (von Blanckenburg et al., 2012) to carbonate landscapes, and performed thorough ground-truthing and testing of assumptions, as this is the first application of the framework for carbonate lithologies. The most important methodological findings are as follows: 1) We amended a sequential extraction step specific for solubilizing total carbonate-bound Be using acetic acid. As this extraction cannot distinguish between secondary and primary carbonate, we employed carbon stable isotopes to obtain the fraction of Be associated with secondary carbonate. We find that >90% of total carbonate-bound Be is bound to secondary carbonate, meaning that distinguishing between secondary and primary carbonate and employing carbon stable isotopes may not be necessary. 2) Using radiogenic strontium isotope ratios we found that about a third of the 9Be contained in secondary carbonate is derived from the dissolution of silicate phases, likely clastic impurities such as clays. These silicate phases also adsorb meteoric 10Be during weathering. The method is thus applicable to pure limestone as well as mixed carbonate-siliciclastic lithologies. 3) Total 9Be concentrations in bedrock are heterogeneous in the Jura, and are potentially controlled by the amount of silicate impurities contained in limestone. Yet the average 9Beparent in summed carbonate- and silicate-bound fractions (0.07 ug/g) is about 9 times lower than values from existing rock databases. In limestones studies, 9Beparent must be thus determined case-by-case on local bedrock. 4) The analysis of partition coefficients Kd for 10Be and 9Be, respectively, and very similar 10Be/9Be ratios show that dissolved Be has equilibrated between reactive (amorphous and crystalline Fe-oxides) and secondary carbonate phases. Secondary carbonate phases are thus part of the reactive Be pool in limestone settings. 5) As in previous studies in silicate lithologies 10Be and 9Be concentrations show pronounced differences between soil and sediment samples that we attribute to grain size dependence and sorting. The 10Be/9Be ratios however cover a remarkably narrow range for all samples, resulting a in narrow range in denudation rates. 6) The fraction of 9Be released by weathering and partitioned into the secondary reactive or dissolved phase serves as a Be-specific proxy for the degree of weathering. 7) The atmospheric depositional flux of 10Be estimated for the Jura mountains from concentrations of dissolved and particulate 10Be and river gauging is about 80% of estimates from independent global GCM-based distribution maps. The GCM estimates thus provide sufficient accuracy. From application of these new principles, weathering and erosion in the French Jura Mountains can be described as follows: The proportion of weathering in total denudation W/D is >0.9, due to the high purity of the limestone that almost completely dissolved except for a small silicate mineral fraction that, however, carries 50% of the bedrock’s 9Be. Resulting 10Be/9Be-derived denudation rates are on average 300 t/km2/yr for soils and 580 t/km2/yr for river sediments. The soil-derived values agree well with previous estimates from gauging data despite their entirely different (decadal vs. millennial) integration time scales. That sediment-derived denudation rates exceed those from soil we attribute to a 30-60% contribution from subsurface bedrock weathering. On a global scale, our data provides the first cosmogenic-based denudation rates for the precipitation (MAP) range of 1200 to 1700 mm/yr under a temperate climate and dense vegetation cover. Previous millennial-scale denudation rates from in situ-36Cl in calcite from less vegetated sites do not exceed 250 t/km2/yr in this precipitation range. With 500-600 t/km2/yr our denudation rates peak at MAP of 1200-1300 mm/yr, and then show a trend of decreasing D with increasing MAP.
Authors
- Wittmann, Hella ;
- Bouchez, Julien ;
- Calmels, Damien ;
- Gaillardet, Jerome ;
- Frick, Daniel ;
- Stroncik, Nicole ;
- ASTER Team ;
- von Blanckenburg, Friedhelm
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Authors
- Ansart, Patrick ;
- Azougui, Abdelkader ;
- Blanchouin, Arnaud ;
- Cordier, Laure ;
- Floury, Paul ;
- Gaillardet, Jerome ;
- Nespoulet, Romane ;
- Tallec, Gaelle
This file contains the dataset used in the publication of Nevers et al. entitled "Landslides as geological hotspots of CO2 to the atmosphere: clues from the instrumented Séchilienne landslide, Western European Alps" published in E-surf Discussions (doi:10.5194/esurf-2020-42) and accepted for publication in E-surf with minor revisions as of Mar. 15, 2021. The dataset remains the same between the two publications.The file is made of three spreadsheets, each corresponding to a particular data table.Tab 1: Major and trace elements concentrations and strontium isotopic composition of rock samples from the Séchilienne slopeTab. 2: Sulfur isotopic composition of bedrock samples from the Séchilienne slopeTab. 3: Chemical and isotopic composition of waters samples of the Séchilienne slope
Authors
- Pierre Nevers ;
- Julien Bouchez ;
- Jérôme Gaillardet ;
- Christophe Thomazo ;
- Laëticia Faure ;
- Catherine Bertrand
This file contains the dataset used in the publication of Nevers et al. entitled "Landslides as geological hotspots of CO2 to the atmosphere: clues from the instrumented Séchilienne landslide, Western European Alps" published in E-surf Discussions (doi:10.5194/esurf-2020-42) and accepted for publication in E-surf with minor revisions as of Mar. 15, 2021. The dataset remains the same between the two publications.The file is made of three spreadsheets, each corresponding to a particular data table.Tab 1: Major and trace elements concentrations and strontium isotopic composition of rock samples from the Séchilienne slopeTab. 2: Sulfur isotopic composition of bedrock samples from the Séchilienne slopeTab. 3: Chemical and isotopic composition of waters samples of the Séchilienne slope
Authors
- Pierre Nevers ;
- Julien Bouchez ;
- Jérôme Gaillardet ;
- Christophe Thomazo ;
- Laëticia Faure ;
- Catherine Bertrand
Sampling large river´s sediment at outlets for cosmogenic nuclide analysis yields mean denudation rates of the sediment producing areas that average local variations in denudation commonly found in small rivers. Using this approach, we measured in situ cosmogenic 26Al and 10Be concentrations in sands of >50 large rivers over a range of climatic and tectonic regimes covering 32% of Earth’s terrestrial surface. River samples were processed in the Helmholtz Laboratory for the Geochemistry of the Earth Surface (HELGES) (von Blanckenburg et al., 2016). 10Be/9Be ratios were measured by Accelerator Mass Spectrometry (AMS) at the University of Cologne and normalized to the KN01-6-2 and KN01-5-3 standards. Denudation rates were calculated using a time-dependent scaling scheme according to Lal/Stone ”Lm” scaling (see Balco et al., 2008) together with a sea level high latitude (SLHL) production rate of 4.13 at/(gxyr) as reported by Martin et al. (2017). Measured in the mineral quartz, the cosmogenic nuclides 26Al and 10Be provide information on how fast Earth´s surface is lowering through denudation. If sediment is however stored in catchments over time spans similar to the nuclides half-lives (being 0.7 Myr and 1.4 Myr for 26Al and 10Be, respectively), the nuclide´s budget is disturbed, and meaningful denudation rates cannot be calculated. The ratio of 26Al/10Be informs us about these disturbances. In 35% of analyzed rivers, we find 26Al/10Be ratios significantly lower than these nuclides´ surface production rate ratio of 6.75 in quartz, indicating sediment storage and burial exceeding 0.5 Myr. We invoke mainly a combination of slow erosion, long transport, and low runoff for these low ratios. In the other 65% of rivers we find 26Al/10Be ratios within uncertainty of their surface production-rate ratio, indicating cosmogenic steady state, and hence meaningful denudation rates can be calculated. For these rivers, we derive a global source-area denudation rate of 140 t/km^2/yr that translates to a flux of 3.10 Gt/yr. By assuming that this sub-dataset is geomorphically representative of the global land surface, we upscale this value to the total surface area for exorheic basins, thereby obtaining a global denudation flux from cosmogenic nuclides of 15.1 Gt/yr that integrates over the past 5 kyr. In Table S1, we provide detailed 10Be nuclide production rates and their correction due to ice shielding and carbonates that are necessary to calculate denudation rates. We provide International GeoSample Numbers (ISGN) for samples used in the analysis, except values that were compiled from published sources. We then compare these denudation rates, converted to sediment fluxes, to published values of sediment fluxes from river load gauging. We find that our cosmogenic nuclide-derived sediment flux value is similar, within uncertainty, to published values from cosmogenic nuclides from small river basins (23 Gt/yr) upscaled using a global slope model, and modern sediment and dissolved loads exported to the oceans (23.6 Gt/yr). In Table S3, we compiled these modern sediment loads and give their references. We also compiled runoff values (mm/yr) from published sources (Table S2) that are used to infer what controls denudation rates. For more details on the sampling and analytical methods, please consult the data description part of this publication.
Authors
- Wittmann, Hella ;
- Oelze, Marcus ;
- Gaillardet, Jerome ;
- Garzanti, Eduardo ;
- von Blanckenburg, Friedhelm
Observational data from ionic chromatography and physico-chemical probes. All data is measured at high-frequency. Data have been collected during CRITEX/EQUIPEX project on the ORACLE observatory (INRAE). These data are free available on the BDOH database (https://doi.org/10.17180/obs.oracle).
Authors
- Ansart, Patrick ;
- Azougui, Abdelkader ;
- Blanchouin, Arnaud ;
- Cordier, Laure ;
- Floury, Paul ;
- Gaillardet, Jérôme ;
- Nespoulet, Romane ;
- Tallec, Gaëlle