Automated Author Profile

Dallin, Bradley

University of Wisconsin–Madison
0000-0002-8580-2816

Current S-Index

2.3

Sum of Dataset Indices for all datasets

Average Dataset Index per Dataset

0.8

Average Dataset Index per dataset

Total Datasets

3

Total datasets for this author

Average FAIR Score

75.6%

Average FAIR Score per dataset

Total Citations

4

Total citations to the author's datasets

Total Mentions

0

Total mentions of the author's datasets

S-Index Interpretation

S-Index Over Time

Cumulative Citations Over Time

Cumulative Mentions Over Time

Datasets

Data for Structural Features of Interfacial Water Predict the Hydrophobicity of Chemically Heterogeneous Surfaces

Scripts, raw and processed data, Jupyter notebooks, and force field files for the simulations performed in: B. C. Dallin, A. S. Kelkar, and R. C. Van Lehn. “Structural Features of Interfacial Water Predict the Hydrophobicity of Chemically Heterogeneous Surfaces.” Chemical Science 2023.

Authors

  • Dallin, Bradley C. ;
  • Kelkar, Atharva S. ;
  • Van Lehn, Reid C.
2 Citations0 Mentions79% FAIR1.1 Dataset Index
10.5281/zenodo.75262542023

Data for Structural Features of Interfacial Water Predict the Hydrophobicity of Chemically Heterogeneous Surfaces

Scripts, raw and processed data, Jupyter notebooks, and force field files for the simulations performed in: B. C. Dallin, A. S. Kelkar, and R. C. Van Lehn. “Structural Features of Interfacial Water Predict the Hydrophobicity of Chemically Heterogeneous Surfaces.” Chemical Science 2023.

Authors

  • Dallin, Bradley C. ;
  • Kelkar, Atharva S. ;
  • Van Lehn, Reid C.
0 Citations0 Mentions79% FAIR0.4 Dataset Index
10.5281/zenodo.75262532023

Dual loop active learning of hydrophobicity of patterned SAMs (Version: 4)

Hydrophobic interactions drive numerous biological and synthetic processes. The materials used in these processes often possess chemically heterogeneous surfaces that are characterized by diverse chemical groups positioned in close proximity at the nanoscale; examples include functionalized nanomaterials and biomolecules like proteins and peptides. Nonadditive contributions to the hydrophobicity of such surfaces depend on the chemical identities and spatial patterns of polar and nonpolar groups in ways that remain poorly understood. Here, we develop a dual-loop active learning framework that combines a fast, reduced-accuracy method (a convolutional neural network) with a slow, higher-accuracy method (molecular dynamics simulations with enhanced sampling) to efficiently predict the hydration free energy, a thermodynamic descriptor of hydrophobicity, for nearly 200,000 chemically heterogeneous self-assembled monolayers (SAMs). Analysis of this data set reveals that SAMs with distinct polar groups exhibit substantial variations in hydrophobicity as a function of their composition and patterning, but the clustering of nonpolar groups is a common signature of highly hydrophobic patterns. Further MD analysis relates such clustering to the perturbation of interfacial water structure. These results provide new insight into the influence of chemical heterogeneity on hydrophobicity via quantitative analysis of a large set of surfaces, enabled by the active learning approach. Paper title: Identifying Nonadditive Contributions to the Hydrophobicity of Chemically Heterogeneous Surfaces via Dual-Loop Active LearningAuthors: Atharva Kelkar, Bradley Dallin, Reid Van LehnDOI: doi.org/10.1063/5.0072385

Authors

  • Kelkar, Atharva ;
  • Dallin, Bradley ;
  • Van lehn, Reid
2 Citations0 Mentions69% FAIR1.1 Dataset Index
10.5061/dryad.41ns1rnft2022