Automated Author ProfileBedoya-Pinto, Amilcar
Instituto de Ciencia Molecular, Universidad de Valencia, C/Catedrático José Beltrán 2, 46980 Paterna, Spain
Bedoya-Pinto, Amilcar
Current S-Index
Sum of Dataset Indices for all datasets
Average Dataset Index per Dataset
Average Dataset Index per dataset
Total Datasets
Total datasets for this author
Average FAIR Score
Average FAIR Score per dataset
Total Citations
Total citations to the author's datasets
Total Mentions
Total mentions of the author's datasets
S-Index Interpretation
The S-Index (Sharing Index) is a comprehensive metric that represents the cumulative impact of all your datasets. It is calculated as the sum of Dataset Index scores across all your claimed datasets.
What it means:
- A higher S-index indicates greater overall impact of your datasets relative to typical datasets in their fields of research
- The S-Index grows as you add more datasets or as existing datasets gain more citations and mentions
- It provides a single number to track your research data impact over time
Current S-Index: 1.1 (sum of 2 datasets Dataset Index scores)
More information here.
S-Index Over Time
Cumulative Citations Over Time
Cumulative Mentions Over Time
Datasets
Single-molecule magnets (SMMs) showing magnetic blocking near or above liquid nitrogen temperature have recently been achieved by inducing exceptionally strong and axial crystal fields via double decker ligands. However, further enhancing the performance at higher temperatures becomes a formidable task. Here we provide an alternative strategy to advance towards this goal by entrapping a single dysprosium(III) ion within a nitrogen-substituted carbon cage. In this structure of Dy@C81N, DyIII is asymmetrically coordinated by one side to a hexagonal carbon ring of the azafullerene, while lacking any coordination ligand on the other side. Despite the very weak crystal field resulting from this very unusual low-coordination environment, this compound exhibits a high blocking temperature (TB, defined as T(t100s)) of 45 K. Its extraordinary magnetic behavior is attributed to the minimal number of vibrations that couple to its spin states, being also responsible for the unusual slow Raman relaxation mechanism observed at high temperatures.
Authors
- Hu, Ziqi ;
- Wang, Yuanyuan ;
- Ullah, Aman ;
- Gutiérrez-Finol, Gerliz M. ;
- Bedoya-Pinto, Amilcar ;
- Gargiani, Pierluigi ;
- Shi, Dier ;
- Yang, Shangfeng ;
- Shi, Zujin ;
- Gaita-Arińo, Alejandro ;
- Coronado, Eugenio
Single-molecule magnets (SMMs) showing magnetic blocking near or above liquid nitrogen temperature have recently been achieved by inducing exceptionally strong and axial crystal fields via double decker ligands. However, further enhancing the performance at higher temperatures becomes a formidable task. Here we provide an alternative strategy to advance towards this goal by entrapping a single dysprosium(III) ion within a nitrogen-substituted carbon cage. In this structure of Dy@C81N, DyIII is asymmetrically coordinated by one side to a hexagonal carbon ring of the azafullerene, while lacking any coordination ligand on the other side. Despite the very weak crystal field resulting from this very unusual low-coordination environment, this compound exhibits a high blocking temperature (TB, defined as T(t100s)) of 45 K. Its extraordinary magnetic behavior is attributed to the minimal number of vibrations that couple to its spin states, being also responsible for the unusual slow Raman relaxation mechanism observed at high temperatures.
Authors
- Hu, Ziqi ;
- Wang, Yuanyuan ;
- Ullah, Aman ;
- Gutiérrez-Finol, Gerliz M. ;
- Bedoya-Pinto, Amilcar ;
- Gargiani, Pierluigi ;
- Shi, Dier ;
- Yang, Shangfeng ;
- Shi, Zujin ;
- Gaita-Arińo, Alejandro ;
- Coronado, Eugenio